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We perform coherent population trapping (CPT) experiments to measure the hyperfine coupling of a single 73GeV to be A∼37 MHz. Furthermore, we identify a rapid nuclear spin diffusion process that occurs when performing CPT and leverage it to realise all-optical, arbitrary nuclear state preparation at timescales approaching ∼1 μs. This is a fundamental step in gaining access to the otherwise difficult to address nuclear spin qudit and paves the way for future research regarding the 73GeV.
Chris Adambukulam,Brett C. Johnson,Andrea Morello, andArne Laucht
"Hyperfine spectroscopy and fast all-optical arbitrary nuclear state preparation of a single 73Ge vacancy in diamond", Proc. SPIE PC12633, Photonics for Quantum 2023, PC126330B (19 July 2023); https://doi.org/10.1117/12.2675865
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Chris Adambukulam, Brett C. Johnson, Andrea Morello, Arne Laucht, "Hyperfine spectroscopy and fast all-optical arbitrary nuclear state preparation of a single 73Ge vacancy in diamond," Proc. SPIE PC12633, Photonics for Quantum 2023, PC126330B (19 July 2023); https://doi.org/10.1117/12.2675865