Recently, we developed a simple, sensitive, and single-beam method for measuring the local nonlinear refraction using a tightly focused laser beam and the Nonlinear Ellipse Rotation (NER) signal. Such configuration allows mapping the nonlinear refraction as a function of depth. The NER signal for pure instantaneous nonlinearity is inversely proportional to the pulse width, which can be shortened or lengthened depending on the sign of the sample’s dispersion and the input pulse chirp and pulse propagation length. However, in materials exhibiting non-instantaneous molecular orientation effects, such as liquids, we have to take into account the effective nonlinear refraction. Hence, here we propose to perform NER measurements in thick and highly dispersive samples, with instantaneous and non-instantaneous refractive nonlinearities, to obtain both the pulse and sample’s parameters, including the nonlinear refraction as a function of the pulse width.
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