Presentation + Paper
12 March 2024 Controlling the pulse width by the sample’s second-order dispersion to study its instantaneous and non-instantaneous nonlinear refractions
R. M. Moysés, E. C. Barbano, L. Misoguti
Author Affiliations +
Abstract
Recently, we developed a simple, sensitive, and single-beam method for measuring the local nonlinear refraction using a tightly focused laser beam and the Nonlinear Ellipse Rotation (NER) signal. Such configuration allows mapping the nonlinear refraction as a function of depth. The NER signal for pure instantaneous nonlinearity is inversely proportional to the pulse width, which can be shortened or lengthened depending on the sign of the sample’s dispersion and the input pulse chirp and pulse propagation length. However, in materials exhibiting non-instantaneous molecular orientation effects, such as liquids, we have to take into account the effective nonlinear refraction. Hence, here we propose to perform NER measurements in thick and highly dispersive samples, with instantaneous and non-instantaneous refractive nonlinearities, to obtain both the pulse and sample’s parameters, including the nonlinear refraction as a function of the pulse width.
Conference Presentation
(2024) Published by SPIE. Downloading of the abstract is permitted for personal use only.
R. M. Moysés, E. C. Barbano, and L. Misoguti "Controlling the pulse width by the sample’s second-order dispersion to study its instantaneous and non-instantaneous nonlinear refractions", Proc. SPIE 12875, Frontiers in Ultrafast Optics: Biomedical, Scientific, and Industrial Applications XXIV, 128750A (12 March 2024); https://doi.org/10.1117/12.3002494
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KEYWORDS
Ultrafast phenomena

Refraction

Dispersion

Pulse signals

Nonlinear optics

Pulsed laser operation

Picosecond phenomena

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