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Excited state absorption spectra of Cr4+-doped garnets and wurtzite-like crystals were measured between 400 nm and 2000 nm. In Cr4+:Y3Al5O12, a strong polarization dependence of the excited state absorption is observed, while it diminishes for Cr4+:Y3Sc0.5Al4.5O12 and is almost not observed in Cr4+:Y3Sc2Ga3O12. FOr Cr4+:LiAlO2 and Cr4+:LiGaO2 the region of the emission is overlapped by excited state absorption and nonlaser oscillation at room temperature is expected.
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Stefan Kueck, S. Hartung, Kenneth L. Schepler, Klaus Petermann, Guenter Huber, "Excited-state absorption and stimulated emission in Cr4+-doped oxide crystals," Proc. SPIE 3176, Tunable Solid State Lasers, (1 November 1997); https://doi.org/10.1117/12.293480